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Quantum effects in dilute adsorption systems

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Title: Quantum effects in dilute adsorption systems
Author: Macrury, Thomas Bernard
Degree Master of Science - MSc
Program Chemistry
Copyright Date: 1967
Subject Keywords Quantum chemistry; Adsorption
Abstract: The adsorption isotherm and the equation of state for the two-dimensional gas are derived from the grand canonical ensemble. Then the quantum statistical equation'of state is developed and applied to the two-dimensional second virial coefficient, B⁽²⁾, and the second gas-surface virial coefficient, B[subscript]AS, We compare theoretically the (12,6) and (12,6,3) potential models for B⁽²⁾. Finally the adsorption data for CH₄, CD₄, H₂ and D₂ on graphite are analysed quantally for the two-dimensional second virial coefficient and the second gas-surface virial coefficient.
URI: http://hdl.handle.net/2429/36546
Series/Report no. UBC Retrospective Theses Digitization Project [http://www.library.ubc.ca/archives/retro_theses/]
Scholarly Level: Graduate

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